and S.K. Ellen MacArthur Foundation. Bars, organized by major regions, show changes for the states. https://www.vitalstrategies.org/resources/excess-mortality-in-brazil-a-detailed-description-of-trends-in-mortality-during-the-covid-19-pandemic/ (2020). Eng. Acrylic acid and derivatives. 109, 57555798 (2009). We performed all demographic analyses in Microsoft Excel version 16.44 and data cleaning and processing in Stata version 15.1 (Stata Corporation) and R version 4.0.0 (2020). Google Scholar. et al. Life cycle assessments (LCA) were performed to assess the cumulative energetic and environmental impacts of producing 1kg of adhesive via our open-loop recycling method. Abbasi, J. Recent efforts to sidestep this degradation using microwaves and added radical initiators led to oligomeric products with 5060% decarboxylation19. Sci. Proposals under this topic must address EU Nature and Biodiversity legislation compliance assurance and access to justice by:- establishing new or, where in place, enhancing existing cross-border, national or regional networks of compliance assurance practitioners or experts; and/or establishing or, where in place, improving professional SEARCH OTHER FUNDING OPPORTUNITIES OR REGISTER TO ACCESS ALL THE INFORMATION AND R&D PROJECTS OPPORTUNITIES IN YOUR AREAS OF INTEREST, Proposals under this topic must address EU Nature and Biodiversity legislation compliance assurance and access to justice by:- establishing new or, where in place, enhancing existing cross-border, national or regional networks of compliance assurance practitioners or experts; and/or establishing or, where in place, improving professional qualifications and training to improve compliance with binding EU legal instruments on nature and biodiversity, through promoting, checking and enforcing compliance, or- applying the polluter pays principle, using a mix of administrative law, criminal law and environmental [], What is This result suggests that most crosslinks had been hydrolyzed within 15h (Supplementary Fig. The COVID-19 pandemic in Brazil: analysis of supply and demand of hospital and ICU beds and mechanical ventilators under different scenarios. We assumed that those dying in a given month from any cause contributed, on average, 0.5/12 person-years, whereas the contribution of survivors was 1/12 person-years. Brazil does not lack a universal healthcare system, a network of community health agents to target vulnerable communities, sufficient data and a capable cadre of researchers tirelessly advancing knowledge and informing policy. United States Environmental Protection Agency (EPA)Office of Land and Emergency Management. Prot. The aim of the project is the conservation of Caretta caretta, in the western Mediterranean basin, from threats related to human disturbance in the nesting sites. Thiounn, T. & Smith, R. C. Advances and approaches for chemical recycling of plastic waste. J. Adhes. The lack of a coordinated, prompt and equitable response informed by science, as well as the promotion of disinformation, have been the hallmark of the current administration27. Moreover, mechanical recycling cannot be used with polymers that do not reversibly melt (e.g., crosslinked polymers). Collias, D. I. et al. S2). 79, 22302244 (2001). We used three approaches to assess changes in life expectancy due to COVID-19. Polym. Second, in contrast to DT19 and DT20, the method based on the difference in life expectancy between 2019 and 2020 makes no assumption about independence of causes of death (that is, that the risks of dying from other causes are unaffected by the addition or elimination of COVID-19 mortality), an assumption that was almost certainly violated during the pandemic. Nature Governance ). Sonication has previously been used to chain-shorten high-molar mass polymers with various backbone architectures31,32, including polyacrylic acid33, and has been used at scale34. U.S. Patent 8404887B2 (March 26, 2013). Experienced Manager with a demonstrated history of working in the computer software industry. Vilseck, J. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. PubMed Central GetScriptingEngine End If If Not IsObject (connection) Then Set connection = application. Innovation Place, CONNECTING Moreover, the life cycle assessments, which utilized soiled diapers as the starting point, demonstrated that these open-loop recycling methods outperform the conventional routes from petroleum-derived feedstocks on nearly every metric, including for the key LCA metrics of global warming potential and cumulative energy demand. Defined and directed strategic marketing and go-to-market plans. A facile and highly efficient strategy for esterification of poly(meth)acrylic acid with halogenated compounds at room temperature promoted by 1,1,3,3-tetramethylguanidine. 2 0 obj CAS 3b). The resulting chain-shortened PAAP&G fragments were then dialyzed to remove excess acid, lyophilized, and then ground into a powder. quizlet cosmetology. performed all wet-lab experimental work under the guidance of A.J.M. <>/Metadata 249 0 R/ViewerPreferences 250 0 R>> When acetic acid was reacted with 2-ethylhexanol/water, we observed a 94% conversion. & Bowe, B. High-dimensional characterization of post-acute sequelae of COVID-19. https://www.ipea.gov.br/portal/index.php?option=com_content&view=article&id=37022&Itemid=448 (2020). The images or other third party material in this article are included in the articles Creative Commons license, unless indicated otherwise in a credit line to the material. Third, for both 2020 and 2021, we calculated life tables based on the addition of COVID-19 mortality to the mortality pattern of 2019 (DT19). 75, 337345 (2002). Use the Previous and Next buttons to navigate the slides or the slide controller buttons at the end to navigate through each slide. Of the gains achieved in e0 in Brazil over 2 decades, 19% were lost due to COVID-19 (Supplementary Table 8). 32, 290299 (2016). . LIFE-2021-SAP-NAT-GOV Nature Governance Each project application under the call must address only one of these topics. Here, chemical transformations are used to convert waste polymers into other value-added materials, delaying their entry into the waste stream. 61, 25842587 (1939). M.C.C. :X"."o:XKw$0/vvDvXK Blackwhite risk differentials in COVID-19 (SARS-COV2) transmission, mortality and case fatality in the United States: translational epidemiologic perspective and challenges. Google Scholar. - Experienced in end-to-end order management process using SAP <br>- More than fourteen (14) years of experience on data analysis, which provides strategic and tactical support to Real Estate documents from various counties in the United States<br>- Self-motivated, results-oriented, and able to work with minimal supervision<br>- Possess proven problem solving abilities and very strong . Our results point to an overall widening of the femalemale gap in e0 of 0.6 years in Brazil (9.1% increase). Heuveline, P. & Tzen, M. Beyond deaths per capita: comparative COVID-19 mortality indicators. Sci. Vaupel, J. W., Villavicencio, F. & Bergeron-Boucher, M.-P. Demographic perspectives on the rise of longevity. volume12, Articlenumber:4524 (2021) State acronyms by region: North: AC=Acre, AP=Amap, AM=Amazonas, PA=Par, RO=Rondnia, RR=Roraima and TO=Tocantins; Northeast: AL=Alagoas, BA=Bahia, CE=Cear, MA=Maranho, PB=Paraba, PE=Pernambuco, PI=Piau, RN=Rio Grande do Norte and SE=Sergipe; Center-West: DF=Distrito Federal, GO=Gois, MT=Mato Grosso and MS=Mato Grosso do Sul; Southeast: ES=Esprito Santo, MG=Minas Gerais, RJ=Rio de Janeiro and SP=So Paulo; South: PR=Paran, RS=Rio Grande do Sul and SC=Santa Catarina. Brazils unified health system: the first 30 years and prospects for the future. Numbers above. Governors in that region imposed the most rigorous measures of physical distancing, in direct opposition to recommendations from the President14. Specifically, using a 2 or 3 step synthetic process, the sodium polyacrylate is converted into a pressure-sensitive adhesive (PSA), which has a significant global market (expected to be $13 billion by 2023) (https://www.alliedmarketresearch.com/pressure-sensitive-adhesives-market). Assuming that death rates would have been equal to 2019 all-cause rates in the absence of COVID-19, COVID-19 deaths in 2021 have already reduced e0 in 2021 by 1.8 years, which is slightly larger than the reduction estimated for 2020 under similar assumptions. Nature and Biodiversity ID LIFE-2021-SAP-NAT-NATURE . Nature Communications (Nat Commun) 29, 233246 (1990). ADS Nat Commun 12, 4524 (2021). Anjeza Beharaj, Ethan Z. McCaslin, Mark W. Grinstaff, Aya Samir, Fatma H. Ashour, Mohamed Bassyouni, Amar K. Mohanty, Feng Wu, Manjusri Misra, Hom N. Sharma, Jeremy M. Lenhardt, Long N. Dinh, Ephraim G. Morado, Mara L. Paterson, Steven C. Zimmerman, Anna M. Duraj-Thatte, Avinash Manjula-Basavanna, Neel S. Joshi, Ainara Sangroniz, Jian-Bo Zhu, Haritz Sardon, Nature Communications Alarifi, A. S. & Aouak, T. Synthesis of acrylic or methacrylic acid/acrylate or methacrylate ester polymers using pervaporation. Slider with three articles shown per slide. T32 AG000037). 4: COVID-19 mortality in 2021 and changes in life expectancy by state and sex. Proc. Also, demographic projections did not account for the pandemic context and might have overestimated population size. To avoid inconsistencies between life tables estimated for 2019 and 2020, we applied the same methodology to 2019. LIFE - Support for applicants (europa.eu) J. Following multiple decrement life table methods previously used to measure the effect of COVID-19 on life expectancy8,16,17, we calculated two additional sets of estimates of life expectancy decline: (1) the difference between 2020 life expectancy estimated above and a scenario in which COVID-19 mortality has been eliminated from 2020 (DT20; Supplementary Tables 3 and 4 and Methods); and (2) the difference between 2019 life expectancy estimated from 2019 death records and a scenario in which 2019 all-cause mortality has been inflated to include COVID-19 mortality (DT19; Supplementary Tables 5 and 6 and Methods). Posta Elettronica Certificata (PEC): protocollo.ispra@ispra.legalmail.it, Kick-off meeting of the projet LIFE-2021-SAP-NAT-NATURE TURTLENEST, https://www.isprambiente.gov.it/en/news/kick-off-meeting-of-the-projet-life-2021-sap-nat-nature-turtlenest, https://www.isprambiente.gov.it/en/news/kick-off-meeting-of-the-projet-life-2021-sap-nat-nature-turtlenest/@@download/image/carretta.png. For e65, the decline in 2021 was estimated at 1.05 years for both sexes (Fig. Boletim Extraordinrio do Observatrio Covid-19 Fiocruz. Nat. For each state and sex, we calculated the difference between the two life tables to estimate reductions in e0 and e65 due to COVID-19 (Supplementary Tables 1 and 2). A summary of findings and implications of these estimates is shown in Table 1. Esterification of polyacrylic acid using alkyl halides under basic conditions had already been reported38. Opening date: 13 July 2021 Deadline: 30 November 2021 Code: LIFE-2021-SAP-NAT-GOV Programme: LIFE - Programme for the Environment and Climate Action Go to the call Objective To contribute to the protection of nature and biodiversity by: Supporting nature and biodiversity policy and legislation compliance assurance, and/or The G at each frequency describes an adhesives ability to dissipate energy. You are using a browser version with limited support for CSS. Created a powerful network of specialist vendors Key qualities and experiences: Project delivery of complicated, multi stream, long-term projects from inception to BAU Business process optimization. Therefore, we estimated the provisional decline in life expectancy in 2021 thus far; this estimate is based on the DT19 method noted earlier but, in this case, adding confirmed 2021 COVID-19 deaths to the deaths expected among those who did not die of COVID-19, who are assumed to be subject to 2019 mortality rates for the remainder of 2021 (Supplementary Table 11). Decrosslinking has been reported using ozonolysis16, though not for the purposes of mechanical recycling. ISSN 2041-1723 (online). 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Chazovachii, P. T., Somers, M., Alfaro, J., McNeil, A. J. J. Mol. Thank you for visiting nature.com. 100th Anniversary of macromolecular science viewpoint: redefining sustainable polymers. https://virological.org/t/first-reported-cases-of-sars-cov-2-sub-lineage-b-1-617-2-in-brazil-an-outbreak-in-a-ship-and-alert-for-spread/706 (2021). Chem. Creton, C. Pressure-sensitive adhesives: An introductory course. One of the pitfalls of diaper recycling pilots is the low demand for recovered diaper materials, which depreciates the environmental potentiality of such endeavors14. . 1)24,25,26. Plots of weight-average molar mass (Mw) versus time and maximum specific energy (wmax) for sonicating PAAP&G at a 2.5% w/v and b 5.0% w/v. JRSvk] T.A., S.G. and S.K. IBGE. THIS GRANT IS CURRENTLY CLOSED. J. Takaya, C. A. et al. SAP Certified with fifteen years of SAP development experience in UK and New Zealand. <> Andrasfay, T. & Goldman, N. Reductions in 2020 US life expectancy due to COVID-19 and the disproportionate impact on the Black and Latino populations. The superstar forward is not taking anything for granted on her return to netball. Chem. M.C.C. Globally, there have been significant efforts towards recycling the components of diapers28. Demography 43, 647657 (2006). To understand why esterification is so favored, we turned to small molecule model systems (Supplementary Information pgs S17S26). sub-programme "Circular economy and quality of life". 15), producing the relatively small estimates of life expectancy decline. Chem. Chem. c, Bivariate choropleth map of the estimated change in e0 and e65 in 2020 based on the difference from life tables calculated for 2019 and 2020 by state. Locations: Colorado; Nevada, Jersey City, NJ; New York City, NY; Ithaca, NY and Westchester County, NY. Anyone you share the following link with will be able to read this content: Sorry, a shareable link is not currently available for this article. We used several data sources to estimate the changes in e0 and e65 due to COVID-19 by state and sex in Brazil. endobj To obtain Correspondence to Chem. First, we obtained mid-year population projections for 20182020 and abridged life tables estimated for 20002020 by state, age and sex from the Brazilian Institute of Geography and Statistics (Instituto Brasileiro de Geografia e Estatstica, or IBGE, in Portuguese) (https://www.ibge.gov.br/en/statistics/social/population/18176-population-projection.html). Brasil, Grandes Regies e Unidades da Federao 2010. in Estudos e Pesquisas. For the base case scenario (absence of COVID-19), we used mortality rates reported in 2019, which we treated as cause-deleted life tables (that is, there were no deaths from COVID-19 in 2019), and applied these to the population at risk to obtain expected deaths in the absence of COVID-19. Teikti paraik ia. projects in line with the objectives of the LIFE Nature and Biodiversity sub-programme but defined in the Call topic LIFE-2021-SAP-NAT-NATURE are excluded. Commercial polymers are ubiquitous, with a global annual production of approximately 368 million metric tons1, with about 75% of plastics disposed of after a single use2. To obtain Three-quarters attack rate of SARS-CoV-2 in the Brazilian Amazon during a largely unmitigated epidemic. A life cycle assessment was used to compare the routes that involved (i) no sonication, (ii) sonication for 1min (2.5% w/v) and (iii) sonication for 2min (5.0% w/v), including the workup steps, and will be described in more detail below. Get the latest from your favourite shows on National Geographic 58, 13471364 (2020). ANDS is a $120M federally funded national infrastructure innovation project to exploit Australia's research data advantage. The LIFE programme is structured in two fields - Environment and Climate Action - and it contributes to these priorities through its four sub-programmes: Environment field: 1. Castro, M.C., Gurzenda, S., Turra, C.M. By submitting a comment you agree to abide by our Terms and Community Guidelines. Mortality due to COVID-19 is estimated to have reduced e0 in the United States by 1.13 years, setting it back to values observed in 2003 (ref. J. Phys. Nmero 30 116 (Instituto Brasileiro de Geografia e EstatsticaIBGE, Diretoria de Pesquisas, Coordenao de Populao e Indicadores Sociais, 2013). The new plastics economy: rethinking the future of plastics & catalyzing action. They might reduce access to and coverage of primary care and increase infant mortality and avoidable deaths. Error bars are derived from an average of two experiments. The authors declare no other competing interests. Percentage loss due to COVID-19 mortality relative to increases in female and male e0 (a) and e65 (b) between 2000 and 2020 by state. An estimated 6.3 billion metric tons of post-consumer polymer waste has been produced, with the majority (79%) in landfills or the environment. As high life expectancies are predominantly in the South region and the lowest are in the North, these results suggest that COVID-19 mortality reproduced regional inequalities, reflecting the pandemics disproportionate burden among vulnerable groups5 but also spatial patterns of COVID-19 spread18. Lpine, L. & Gilbert, R. Thermal degradation of polyacrylic acid in dilute aqueous solution. Therefore, our estimates would not be seriously affected by missing deaths unless a different pattern of errors emerges in 2020. D.I.C., M.I.J., and E.N.G.M. Chem. Silveira, M. F. et al. "Climate action". volume27,pages 16291635 (2021)Cite this article. These results suggest that the substrate hydrophobicity also favors conversion to the ester. 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S3). Lines represent changes for Brazil. Prod. Coates, G. W. & Getzler, Y. D. Y. L. Chemical recycling to monomer for an ideal, circular polymer economy. Rede PENSSAN. The authors thank Procter and Gamble (P&G) for supporting this work, as well as Ryan Hayes and Jonah Vilseck for assisting with simulations, Edwin Zishiri for assisting with synthesis, Gary Gilbertson, Bill Begley, and Yiping Sun for performing SEC on the PSAs, and Prof. Brian Love for his intellectual contributions. https://www.fatersmart.com/ - (Accessed May 1, 2021). Overall, the viscoelastic properties of the synthesized PSAs suggest they would be useful for applications such as removable general-purpose adhesives, including tapes, bandages, and sticky notes. J. Org. Cancer diagnosis in Brazil in the COVID-19 era. Science 372, 815821 (2021). Briefly, nonamers of polyacrylic acid were used as a model system along withbutanol Comparison of the reaction free energies was made between the first esterification and the final esterification. The change in the Helmholtz free energy of esterification for these two steps (A) was found to be 0.70.1kcal/mol. Because this recycling method should be amenable to waste polymer as the feedstock, it offers a more sustainable alternative to diaper disposal in a landfill or incineration. We calculated nRx, the age-specific and sex-specific ratio of deaths from all causes other than COVID-19 to deaths inclusive of COVID-19. In the first 4 months of 2021, COVID-19 deaths represented 107% of the total 2020 figures. Excitingly, a viable central region pressure-sensitive adhesive is accessible without any sonication. Article J. Appl. State acronyms by region: North: AC=Acre, AP=Amap, AM=Amazonas, PA=Par, RO=Rondnia, RR=Roraima and TO=Tocantins; Northeast: AL=Alagoas, BA=Bahia, CE=Cear, MA=Maranho, PB=Paraba, PE=Pernambuco, PI=Piau, RN=Rio Grande do Norte and SE=Sergipe; Center-West: DF=Distrito Federal, GO=Gois, MT=Mato Grosso and MS=Mato Grosso do Sul; Southeast: ES=Esprito Santo, MG=Minas Gerais; RJ=Rio de Janeiro and SP=So Paulo; South: PR=Paran, RS=Rio Grande do Sul and SC=Santa Catarina. Degrad. Surprisingly, even when excess H2O was intentionally added (3 equiv), high conversions were still observed (Supplementary Information pgs S15S16). and C.M.T. Lotta, G., Wenham, C., Nunes, J. LIFE-2021-SAP-NAT-GOV Nature Governance Standard Action Projects (SAPs) Strategic Nature Projects (SNAPs) SNAPs: (1)target the implementation of the Prioritised Action Frameworks (PAF) other plans or strategies adopted at international, national, regional or multiregional level by nature In Amazonas, male e65 was estimated to decline by 20% from 2019 to 2020. Al-Aly, Z., Xie, Y. Cite this article. We estimated a reduction of 1.31 years in e0 from 2019 to 2020 (Fig. 5)49,50. 1, 46 (2017). <> are employees at P&G. H2SO4 with heating (Fig. Due to these challenges, the focus has been on re-use of recovered materials, rather than recycling; for example, the recovered superabsorbent polymers have been explored for enhancing the water retention properties of soil21,22. CAS We did not make any corrections for the under-registration of deaths. Preparation of pressure sensitive adhesives from post-consumer superabsorbent polymers. Nat Med 27, 16291635 (2021). a, Ratio of COVID-19 deaths reported in 2021 (January-April) to those reported in 2020 (%). What it lacks is leadership commitment to save lives. Previous studies used this approach to estimate life tables in the presence of COVID-19 (refs. For example, high degrees of esterification were observed via 1H NMR spectroscopy when using only 5 equiv. A life cycle assessment was used to compare the routes that involved (i) no sonication, (ii) sonication for 1 min (2.5% w/v) and (iii) sonication for 2 min (5.0% w/v), including the workup steps,. For example, the 1918 influenza pandemic was estimated to have reduced e0 in the United States by 712 years7. Google Scholar. Lancet Glob. Catal. (Wiley-VCH Verlag GmbH & Co, Weinheim, 2020). Nuzzo, J. 1a, Supplementary Table 1 and Methods), with a larger drop for males (1.57 years) than females (0.95 years). Genomics and epidemiology of a novel SARS-CoV-2 lineage in Manaus, Brazil. J. Environ. Castro, M. C. et al. La Commissione europea ha pubblicato i primi bandi del programma LIFE 2021-2027 per l' ambiente, il clima e l' energia . Fornof, A. R. et al. 5). 127, 289301 (2016). Biochem. Article https://doi.org/10.1053/j.seminoncol.2020.12.002 (2021). In any recycling effort, it is essential that a life cycle assessment27 is performed to determine the energy and environmental costs. Single phase. Anyone you share the following link with will be able to read this content: Sorry, a shareable link is not currently available for this article. The materials, equipment, synthetic methods, as well as all processed data generated in this study are provided in the Supplementary Information file. All environmental data were gathered from experiments, literature, or the ecoinvent database (version 3.5)51, and implemented in SimaPro v. 9.0.0.4850, as described in detail within the Supporting Information (Supplementary Information pgs S36S41). We also thank Prof. Charlie Brooks for providing GPU computing resources. of 2-ethylhexanol and H2SO4 as a catalyst (Fig. #n$dA"yTtM nTv_J{Bf25X1E[B Y@V(//G0g4_fc_Cv;`& ,. Palloni, A., Pinto, G. & Beltrn-Snchez, H. Two centuries of mortality decline in Latin America: from hunger to longevity. http://olheparaafome.com.br/VIGISAN_Inseguranca_alimentar.pdf (2021). Google Scholar. The magnitude of the COVID-19 death toll was not homogenous across states and was associated with the pattern of spread18. You can alreadyfind all information and documentation needed at theFunding & Tenders Portal, includingthe call text and application forms. Life Cycle Assess. Under ultrasound, solvodynamic shear forces cleave polymer chains into shorter fragments while maintaining the polymers chemical identity. Here, we assumed that individuals who did not die of COVID-19 in the first 4 months of 2021 would be subject to the 2019 age group-specific and sex-specific mortality rates.